形状记忆高分子材料的网络结构化设计和性能研究

李兴建; 王亚茹; 郑朝晖; 丁小斌; 彭宇行

doi:10.7536/PC130126

化学进展 ›› 2013, Vol. 25 ›› Issue (10) :1726-1738 DOI: 10.7536/PC130126

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形状记忆高分子材料的网络结构化设计和性能研究

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Structural Design and Property Study of Shape Memory Polymer Network

Li Xingjian^1,2, Wang Yaru^1,2, Zheng Zhaohui¹, Ding Xiaobin¹, Peng Yuxing¹

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摘要

形状记忆聚合物是一种可以响应外界刺激,并调整自身状态参数,从而回复到预先设定状态的一种智能高分子材料。它是智能高分子材料研究、开发和应用的一个新热点。在智能纺织材料、生物医用材料、航空航天技术等领域显示了极为广阔的应用前景。为了使形状记忆聚合物材料在这些领域具有更加实际和广泛的应用,通常要求这些材料要有更高的固定率和回复率、更快的回复速度、优异的机械性能和良好的性能可控性。通常情况下材料的结构决定其性能,因此形状记忆聚合物的结构化设计是一个非常值得探讨的话题。本文从网络结构化设计的角度综述了基于互穿网络结构、AB型网络结构、规整网络结构、“互锁”网络拓扑结构设计的形状记忆高分子材料的研究进展,分别介绍了这些材料的结构和性能的关系、特点及其潜在应用。最后,对具有网络结构形状记忆高分子材料的发展方向和应用前景进行了展望。

Abstract

Shape memory polymers (SMPs) are a promising class of intelligent polymer materials that have the ability to recover the permanent shape in a predefined way from the temporary shape in response to external stimuli. SMPs have become a new hot spot in the field of smart materials and have shown many potential applications in various fields, such as smart textile materials, biomedical materials, aerospace technology, and so on. In order to better utilize SMPs in these fields, high recovery rate and fixed rate, excellent mechanical properties, fast response speed, and good adjustable performance are required. Generally, the properties are mainly determined by the intrinsic structure, and the design of SMPs with novel structure has become a worthy topic. In this review, the progress in SMPs design based on the network structure is summarized systematically, including the relationship between their structure and properties, characteristics and potential applications, focusing on the design of SMP materials with interpenetrating network structure, AB network structure, homogenous network structure, topological structure of interlocked network. Finally, the future developments and applications of SMPs with the network structure are prospected.

Contents
1 Introduction
2 Design of SMPs based on interpenetrating network structure
3 Design of SMPs based on AB network structure
4 Design of SMPs based on homogenous network structure
4.1 Design of SMPs based on homogenous network with star structure
4.2 Design of SMPs based on homogenous network structure with nanoparticle netpoints
5 Design of SMPs based on topological structure of interlocked network
6 Conclusion and outlook

关键词

形状记忆 / 互穿网络结构 / AB型网络结构 / 规整网络结构 / “互锁”网络拓扑结构

Key words

shape memory / interpenetrating network structure / AB network structure / homogenous network structure / topological structure of interlocked network

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李兴建, 王亚茹, 郑朝晖, 丁小斌, 彭宇行. 形状记忆高分子材料的网络结构化设计和性能研究[J]. 化学进展, 2013, 25(10): 1726-1738 DOI:10.7536/PC130126

Li Xingjian, Wang Yaru, Zheng Zhaohui, Ding Xiaobin, Peng Yuxing. Structural Design and Property Study of Shape Memory Polymer Network[J]. Progress in Chemistry, 2013, 25(10): 1726-1738 DOI:10.7536/PC130126

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Received	Published	Revised
2013-01-01	2013-11-12	2013-03-01
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2013-07-18

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