聚（3，4-乙撑二氧噻吩）（PEDOT）作为一种成膜性好、热稳定性高、电导率可调且廉价的透明导电高分子材料，在多种能量转换和储存器件中有着诱人的应用前景。然而，较低的电导率等因素制约了基于PEDOT组装的各类器件的实际性能。本文首先简述了PEDOT薄膜的基本性质、常用的化学与物理制备途径以及提高电导率的几种方式，随后综述了PEDOT以及PEDOT和其他物相构成的复合结构在包括太阳能电池、发光二极管、电致变色器件和超级电容器等器件中的应用的最新进展。其中，不仅阐述了PEDOT基材料在上述器件中所起的作用，还详细介绍了针对不同器件对PEDOT基材料的要求，研究人员提出的PEDOT基材料的设计思路，包括设计具有特定微观形貌的PEDOT薄膜、对PEDOT薄膜的电导率、功函数和透光度等进行调控以及将PEDOT和碳材料、金属纳米颗粒、金属氧化物等其他物相进行复合。最后指出了目前在PEDOT基电极材料的研究中面临的挑战，并对该材料的研究前景进行了展望。
As a kind of low-cost transparent conductive material with good film-forming properties, high thermal stability and tunable conductivity, poly(3,4-ethylenedioxythiophene)(PEDOT) has exhibited attractive applications in various energy conversion and storage devices. However, the performances of these devices are restricted by some drawbacks of PEDOT, mainly its low conductivity. In this review, firstly the basic properties, commonly adopted chemical and physical approaches for synthesizing PEDOT films and several ways to improve their conductivity are briefly introduced. Then the latest research progresses of devices including solar cells, light-emitting diodes, electrochromic devices and supercapacitors assembled by PEDOT and PEDOT-based composited materials are reviewed. In addition to elucidating the roles of PEDOT-based materials played in the aforementioned devices, the design ideas of PEDOT-based materials proposed by researchers for fulfilling the requirements of different devices are introduced in detail. The ideas include designing PEDOT films with specific microstructures, modulating the conductivity, work function, optical transparency and other properties of PEDOT, and coupling PEDOT with other active materials such as carbon materials, metal nanoparticles and metal oxides. Finally, the challenges nowadays in the studying of PEDOT-based electrode materials are pointed out, and the prospect of these materials is proposed.
Contents
1 Introduction
2 Preparation and modification of PEDOT based electrode materials
2.1 Preparation of PEDOT based electrode materials
2.2 Modification of PEDOT based electrode materials
3 Applications of PEDOT based electrode materials
3.1 Solar cells
3.2 Light-emitting diodes
3.3 Electrochromic devices
3.4 Supercapacitors
3.5 Other devices
3.6 Working mechanisms of PEDOT based electrode materials
4 Conclusion
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