催化膜的限域机理及其应用

卢娜; 孟宪谭; 梁明; 梁斌; 李留忠

doi:10.7536/PC20260411

化学进展 ›› :0- DOI: 10.7536/PC20260411

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催化膜的限域机理及其应用

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摘要

催化膜是耦合催化反应和膜分离过程的新型膜催化反应器，在水处理过程中可以连续实现难降解污染物的结构转化及矿化。催化膜限域通道的构建及膜孔内限域机理的理解对高性能催化膜的设计和精准应用具有重要意义。本文介绍了不同维度限域通道的构筑方法，并深入分析了限域效应通过三个相互关联的机制来提高催化膜性能：（i）通过提升氧化剂的活化效率、转变氧化剂的活化路径来实现催化效率的跃升，（ii）通过界面浓差极化、尺寸筛分、孔内扩散-反应等过程来强化传质，（iii）通过在限域通道内进行物理封装和微环境调控来增强催化剂的稳定性。在上述理论基础上，总结了催化膜在处理难降解污染物领域的应用，并延伸出限域催化膜在高附加值化合物合成等前沿领域的应用。最后综合分析了限域催化膜在当前面临的挑战与研究热点，并展望了未来需要着重关注的研究方向。

Abstract

Catalytic membranes, which integrate catalytic reactions with membrane separation processes, represent an innovative type of membrane catalytic reactor capable of continuously facilitating the structural transformation and mineralization of refractory pollutants. The rational design and effective deployment of high-performance catalytic membranes hinge critically on the deliberate engineering of confined catalytic nanochannels and a mechanistic understanding of confinement effects within membrane pores. This review introduces the fabrication strategies for confinement channels across diverse dimensional architectures, and critically analyzes how confinement effect enhances catalytic membrane performance through three interrelated mechanisms: (i) boosting catalytic efficiency by improving oxidant activation kinetics and steering alternative activation pathways; (ii) accelerating mass transfer via interfacial concentration polarization, size exclusion effects, and coupled intraporous diffusion-reaction dynamics; and (iii) augmenting catalyst stability through physical encapsulation and microenvironmental regulation within confined domains. Building upon these fundamental insights, we comprehensively survey applications of catalytic membranes in the degradation of recalcitrant pollutants and further highlight emerging applications of confined catalytic membranes in value-added chemical synthesis. Finally, we identify key scientific and technical challenges confronting the field, and propose priority research directions in the future.

关键词

催化膜 / 限域效应 / 传质 / 水处理 / 化学品合成

Key words

catalytic membrane / confinement effect / mass transfer / water treatment / chemical synthesis

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卢娜, 孟宪谭, 梁明, 梁斌, 李留忠. 催化膜的限域机理及其应用[J]. 化学进展, , (): 0 DOI:10.7536/PC20260411

Na Lu, Xiantan Meng, Ming Liang, Bin Liang, Liuzhong Li. Progress in Chemistry 0 DOI:10.7536/PC20260411

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2026-04-09	2026-07-24	2026-06-17
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